On the role of coupling in mode selective excitation using ultrafast pulse shaping in stimulated Raman spectroscopy

Details On the role of coupling in mode selective excitation using ultrafast pulse shaping in stimulated Raman spectroscopy On the role of coupling in mode selective excitation using ultrafast pulse shaping in stimulated Raman spectroscopy

2004-05-03

arxiv.org/abs/physics/0405011v1

Physics

Chemical Physics

7 pages, 4 figures

Scientific paper

10.1063/1.1774985

The coherence of two, coupled two-level systems, representing vibrational modes in a semiclassical model, is calculated in weak and strong fields for various coupling schemes and for different relative phases between initial state amplitudes. A relative phase equal to $\pi$ projects the system into a dark state. The selective excitation of one of the two, two-level systems is studied as a function of coupling strength and initial phases.

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