On the application of Canonical Perturbation Theory up to the dissociation threshold

Details On the application of Canonical Perturbation Theory up to the dissociation threshold On the application of Canonical Perturbation Theory up to the dissociation threshold

2010-01-06

arxiv.org/abs/1001.0835v1

Chemical Physics Letters 412 (2005) 200-205

Physics

Chemical Physics

Scientific paper

10.1016/j.cplett.2005.06.115

We investigate a model system consisting of a Morse oscillator strongly
coupled to a doubly-degenerate bending degree of freedom and show that
Canonical Perturbation Theory is able to provide a fairly precise, though not
exact, approximation of the Hamiltonian up to the dissociation threshold.
Quantum mechanical results and classical ones are discussed in this Letter.

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