Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas

Details Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas Nonperturbative modeling of fifth-order coherent multidimensional spectroscopy in light harvesting antennas

Feb 2011

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2011njph...13b5024b&link_type=abstract

New Journal of Physics, Volume 13, Issue 2, pp. 025024 (2011).

Physics

2

Scientific paper

Recent advances in coherent multidimensional spectroscopy have boosted interest in exciton coherences in light harvesting complexes. We present nonperturbative calculations of two-dimensional (2D) electronic spectroscopy from a fifth-order phase-matching direction. The calculations show clear patterns that correspond to the electronic structure of one- and two-exciton manifolds of a Fenna-Matthews-Olsson light harvesting complex. Such signals can provide new information about the coherent properties of antenna pigment protein complexes.

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