Physics – Computational Physics
Scientific paper
2007-08-21
Phys. Rev. Lett. 100, 116403 (2008)
Physics
Computational Physics
10pages, 4 figures
Scientific paper
10.1103/PhysRevLett.100.116403
Nonlinear dynamics of photoinduced cooperative phenomena is studied by numerical calculations on a model of molecular crystals. We found that the photoinduced nucleation process is triggered only when certain amount of excitation energy is supplied in a narrow part of the system, i.e., there exists a smallest cluster of excited molecules which makes the nucleation possible. As a result, the portion of the cooperatively converted molecules is nonlinearly dependent on the photoexcitation strength, which has been observed in various materials.
Ishida Kunio
Nasu Keiichiro
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