Nonlinear Optical Spectroscopy of Excited States in Polyfluorene

Details Nonlinear Optical Spectroscopy of Excited States in Polyfluorene Nonlinear Optical Spectroscopy of Excited States in Polyfluorene

2006-10-10

arxiv.org/abs/physics/0610074v1

Physics

Optics

20 pages, 6 figures, 1 table

Scientific paper

We used a variety of nonlinear optical (NLO) spectroscopies to study the singlet excited states order, and primary photoexcitations in polyfluorene; an important blue emitting p-conjugated polymer. The polarized NLO spectroscopies include ultrafast pump-probe photomodulation, two-photon absorption, and electroabsorption. For completeness we also measured the linear absorption and photoluminescence spectra. We found that the primary photoexcitations in polyfluorene are singlet excitons.

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