Multiple Ionization of Rare Gas Atoms Irradiated with Intense VUV Radiation

Physics – Optics

Scientific paper

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Multiphoton Ionization And Excitation To Highly Excited States, Nonlinear Optics

Scientific paper

The interaction of intense vacuum-ultraviolet radiation from a free-electron laser with rare gas atoms is investigated. The ionization products of xenon and argon atomic beams are analyzed with time-of-flight mass spectroscopy. At 98nm wavelength and ˜1013 W/cm2 multiple charged ions up to Xe6+ (Ar4+) are detected. From the intensity dependence of multiple charged ion yields the mechanisms of multiphoton processes were derived. In the range of ˜1012 1013 W/cm2 the ionization is attributed to sequential multiphoton processes. The production of multiple charged ions saturates at 5 30times lower power densities than at 193 and 564nm wavelength, respectively.

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