Modeling of growth and evaporation effects on the extinction of 1.0-micron solar radiation traversing stratospheric sulfuric acid aerosols

Physics – Optics

Scientific paper

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Aerosols, Atmospheric Attenuation, Atmospheric Models, Infrared Absorption, Stratosphere, Sulfuric Acid, Water Vapor, Ambient Temperature, Atmospheric Moisture, Environment Models, Evaporation, Particle Size Distribution, Solar Radiation

Scientific paper

The effects of growth and evaporation of stratospheric sulfuric acid aerosols on the extinction of solar radiation traversing such an aerosol medium are reported for the case of 1.0-micron solar radiation. Modeling results show that aerosol extinction is not very sensitive to the change of ambient water vapor concentration, but is sensitive to ambient temperature changes, especially at low ambient temperatures and high ambient water vapor concentration. A clarification is given of the effects of initial aerosol size distribution and composition on the change of aerosol extinction due to growth and evaporation processes. It is shown that experiments designed to observe solar radiation extinction of aerosols may also be applied to the determination of observed changes in aerosol optical properties, environmental parameters, or the physical and optical characteristics of sulfate aerosols.

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