Measuring the quantum efficiency of single radiating dipoles using a scanning mirror

Physics – Optics

Scientific paper

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4 pages, 4 figures

Scientific paper

10.1103/PhysRevLett.95.063003

Using scanning probe techniques, we show the controlled manipulation of the radiation from single dipoles. In one experiment we study the modification of the fluorescence lifetime of a single molecular dipole in front of a movable silver mirror. A second experiment demonstrates the changing plasmon spectrum of a gold nanoparticle in front of a dielectric mirror. Comparison of our data with theoretical models allows determination of the quantum efficiency of each radiating dipole.

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