Low-temperature dynamical simulation of spin-boson systems

Details Low-temperature dynamical simulation of spin-boson systems Low-temperature dynamical simulation of spin-boson systems

1994-11-09

arxiv.org/abs/chem-ph/9411006v1

Physics

Chemical Physics

Phys. Rev. B (in press), 28 pages, 6 figures

Scientific paper

10.1103/PhysRevB.50.15210

The dynamics of spin-boson systems at very low temperatures has been studied using a real-time path-integral simulation technique which combines a stochastic Monte Carlo sampling over the quantum fluctuations with an exact treatment of the quasiclassical degrees of freedoms. To a large degree, this special technique circumvents the dynamical sign problem and allows the dynamics to be studied directly up to long real times in a numerically exact manner. This method has been applied to two important problems: (1) crossover from nonadiabatic to adiabatic behavior in electron transfer reactions, (2) the zero-temperature dynamics in the antiferromagnetic Kondo region 1/2

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