Is UV laser induced fluorescence a method to monitor tropospheric OH

Details Is UV laser induced fluorescence a method to monitor tropospheric OH Is UV laser induced fluorescence a method to monitor tropospheric OH

Nov 1980

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1980georl...7..905o&link_type=abstract

Geophysical Research Letters, vol. 7, Nov. 1980, p. 905-908. Deutsche Forschungsgemeinschaft

Physics

Optics

3

Atmospheric Chemistry, Fluorescence, Hydroxyl Radicals, Laser Induced Fluorescence, Laser Spectroscopy, Troposphere, Ultraviolet Lasers, Atmospheric Optics, Ozone, Photolysis, Vertical Distribution

Scientific paper

Calculations are presented that show the significant interference of laser-generated OH in ambient air with tropospheric OH if the laser-induced fluorescence (LIF) technique is used. A comparison of measurements with results of calculations indicates that the measured tropospheric OH concentration is within the order of magnitude of laser-generated OH. It seems doubtful that the LIF method using 282-nm radiation can be successfully employed for the probing of OH in the troposphere. The main difficulty involves high O(1D) production from the probing laser radiation.

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