Physics – Chemical Physics
Scientific paper
2010-07-15
Phys. Rev. A 83, 023405 (2011)
Physics
Chemical Physics
13 pages, 10 figures
Scientific paper
10.1103/PhysRevA.83.023405
We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show pronounced asymmetries perpendicular to the direction of the molecular electric dipole moment. These findings are explained by a tunneling model invoking the laser-induced Stark shifts associated with the dipoles and polarizabilities of the molecule and its unrelaxed cation. The focus of the present article is to understand the strong-field ionization of one-dimensionally-oriented polar molecules, in particular asymmetries in the emission direction of the photoelectrons. In the following article (Phys. Rev. A 83, 023406 (2011)) the focus is to understand strong-field ionization from three-dimensionally-oriented asymmetric top molecules, in particular the suppression of electron emission in nodal planes of molecular orbitals.
Abu-samha Mahmoud
Dimitrovski Darko
Filsinger Frank
Holmegaard Lotte
Kalhøj Line
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