Ion-ion recombination and ion-pair formation processes in alkali-hydrogen diatomic systems

Physics – General Physics

Scientific paper

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Alkali Metals, Diatomic Molecules, Hydrogen, Ion Recombination, Ionic Reactions, Ionization Cross Sections, Electron Transitions, Metal-Gas Systems, Molecular Excitation, Pair Production, Reaction Kinetics

Scientific paper

The mutual neutralization and ion-pair-formation reactions in alkali-hydrogen diatomic systems are investigated in the low-energy region. The ionic-covalent exchange interaction in these systems at the diabatic curve crossings is calculated by the Landau-Herring method. The cross sections and reaction-rate coefficients of these reactions are calculated using the Landau-Zener theory, modified to include the underbarrier transitions and the effects of the variation of coupling interaction within the transition zone. For Cs-H system, the calculated recombination and ion-pair-formation cross sections are compared with the existing theoretical calculations and experimental data.

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