Physics
Scientific paper
Jun 2010
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2010mss..confewj10c&link_type=abstract
"International Symposium On Molecular Spectroscopy, 65th Meeting, Held 21-25 June, 2010 at Ohio State University. http://molspec
Physics
Radicals And Ions
Scientific paper
Highly fluxional H_5^+ and D_5^+ ions are generated via arc discharge in a pulsed supersonic expansion source and analyzed by infrared photodissociation spectroscopy. A breakdown in the harmonic approximation because of the delocalized and highly anharmonic shared-proton stretch mode has caused uncertainty with previous attempts by Lee and coworkers to assign the peaks. An improvement in quality of the spectra along with good agreement with frequencies from a new fixed-node diffusive Monte Carlo calculation method help assign the peaks to their corresponding vibrational modes.
Bandyopadhyay Bijoy
Bastiaan B. J.
Bowman Joel M.
Carter Scott
Cheng Tai-Chung
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