Hole-burning spectroscopy and relaxation dynamics of amorphous solids at low temperatures

Physics

Scientific paper

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Amorphous Materials, Hole Burning, Low Temperature Physics, Optical Emission Spectroscopy, Relaxation (Mechanics), Absorption Spectra, Normal Density Functions, Temperature Dependence, Time Dependence

Scientific paper

The magnitude and temperature dependence of most of the properties of amorphous solids are anomalous at very low temperatures (less than about 1 Kelvin). Phonon-assisted tunneling of a distribution of glassy bistable configurations, or two-level systems, can account for these anomalies. A unified understanding of the low-temperature properties is required for an understanding of the glassy state. Persistent nonphotochemical hole burning of impurity optical transitions allows a glass state to be produced that is thermally inaccessible to the preburn state, and that allows the probing of tunneling dynamics on time scales that range between picoseconds and days. These data combined with recently obtained distribution functions for the two-level systems offer new insights into the tunneling dynamics.

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