High-resolution spectroscopy of the v2 = 2 a <-- v2 = 1 s band of 14NH3

Details High-resolution spectroscopy of the v2 = 2 a <-- v2 = 1 s band of 14NH3 High-resolution spectroscopy of the v2 = 2 a <-- v2 = 1 s band of 14NH3

Jun 1986

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1986jmosp.117..317s&link_type=abstract

Journal of Molecular Spectroscopy, Volume 117, Issue 2, p. 317-330.

Physics

20

Scientific paper

Twenty-one transitions of the v2 = 2 a <-- v2 = 1 s hot band of 14NH3 have been observed by an infrared microwave sideband laser spectrometer with an absolute accuracy of 0.00002 cm-1. One hundred and seventeen transitions of the band have been obtained by a Fourier transform infrared spectrometer at a resolution of 0.005 cm-1. A weighted least-squares analysis of these data has been carried out to yield 17 molecular parameters for the v2 = 2 a state. These parameters reproduce the experimental frequencies with a root mean square deviation of 0.000123 cm-1. To calculate the frequencies to this accuracy it was necessary to take into account the Δ(K - l) = +/-3 interaction between the v2 = 2 a and v4 = 1 a states.

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