High-order Harmonic Generation in a Time-integrated Quantum Transition Picture

Details High-order Harmonic Generation in a Time-integrated Quantum Transition Picture High-order Harmonic Generation in a Time-integrated Quantum Transition Picture

2008-11-13

arxiv.org/abs/0811.2092v1

Physics

Atomic Physics

5 figures, 5 pages

Scientific paper

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated quantum transition picture. Our full-quantum simulations reveal that continuum electrons with a broad energy distribution contribute equally to one harmonic and the excited state also plays an important role in the molecular HHG. These results imply a laser-intensity-dependent picture of intramolecular interference in the HHG.

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