Helium Nanodroplet Isolation Spectroscopy Using AN External Cavity Quantum Cascade Laser

Physics

Scientific paper

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Matrix/Condensed Phase

Scientific paper

A mode-hop free tunable external cavity quantum cascade laser (Daylight Solutions) is used to probe the vibrational dynamics of helium solvated H_{2}O and NO_{2} monomers and dimers. The demonstrated high output power and mode-hop free tuning of the laser in combination with a multipass cell and bolometric detection allow for high resolution spectroscopy studies of helium solvated molecules between 10 and 5 μm.

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