Green plants: A terrestrial sink for atmospheric CH3Br

Physics

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Atmospheric Composition And Structure: Biosphere/Atmosphere Interactions, Atmospheric Composition And Structure: Chemical Kinetic And Photochemical Properties, Atmospheric Composition And Structure: Troposphere-Composition And Chemistry

Scientific paper

Methyl bromide is reactively removed from air by the foliage of all 9 herbaceous, 18 deciduous, and 12 coniferous plants we have tested, in a process that appears enzymatic. Excised plant leaves yielded removal rates directly proportional to leaf surface area and first-order in CH3Br concentration from 10 ppmv to 500 pptv, the current limit of our experimental technique. Observed rate constants for different plants vary within a factor of about 100 with a lower value of 1×10-3hr-1cm-2 in systems where the rate is not diffusion limited. This sink for atmospheric CH3Br could be significant in calculations of the global methyl bromide budget.

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