Fourier transform detection of laser-induced fluorescence from the CCN free radical

Details Fourier transform detection of laser-induced fluorescence from the CCN free radical Fourier transform detection of laser-induced fluorescence from the CCN free radical

Mar 1987

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1987jchph..86.3078b&link_type=abstract

Journal of Chemical Physics (ISSN 0021-9606), vol. 86, March 15, 1987, p. 3078-3081. Navy-supported research.

Physics

Chemical Physics

17

Cyano Compounds, Fourier Transformation, Free Radicals, Laser Induced Fluorescence, Vibrational Spectra, Laser Spectroscopy, Spin-Orbit Interactions

Scientific paper

A technique of high-resolution Fourier transform spectroscopy in which a bandpass filter blocks scattered laser light is used to detect the laser-induced fluorescence spectrum of the CCN free radical. Only emission from excited vibrational levels of the ground state was observed, and five bands were rotationally analyzed, yielding frequencies for the two stretching modes v1 and v3. The omega2 value determined is in good agreement with the value of Merer and Travis (1965), while the determined size of the Renner-Teller interaction, giving epsilon of 0.410, is slightly different due to their neglect of the small contribution from the gk11 parameter.

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