Four Wave Mixing Spectroscopy at the Interface Between the Time and Frequency Domains

Details Four Wave Mixing Spectroscopy at the Interface Between the Time and Frequency Domains Four Wave Mixing Spectroscopy at the Interface Between the Time and Frequency Domains

2009-07-21

arxiv.org/abs/0907.3625v1

Physics

Optics

24 page article with 4 figures

Scientific paper

Combined spectrally and time resolved measurements provide information not otherwise available if performed in either domain alone. We demonstrate a new approach to Four Wave Mixing spectroscopy, where spectral selectivity is achieved by phase matching filtering without a spectrometer, and the time resolved signal is obtained within a single pulse and without mechanically scanning any delays. We analyze the Degenerate Four Wave Mixing signal, and show that a counter-rotating Feynman diagram not previously considered is necessary in order to understand the measured frequency and time resolved spectrograms.

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