Physics
Scientific paper
Aug 1990
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1990rspta.332..223g&link_type=abstract
Philosophical Transactions: Physical Sciences and Engineering, Volume 332, Issue 1625, pp. 223-243
Physics
24
Scientific paper
Recently, the rapid dissociation dynamics of mercury diiodide has been studied by femtosecond transition-state spectroscopy (FTS). Such experiments provide a real-time picture of wave packet motions in two dissociation channels associated with the iodine atomic product in its ground and spin-orbit excited states. We present here a two-dimensional quantum mechanical treatment of the FTS experiment, which allows us to discuss the salient features of the wave packet motion and product state distribution. Possible refinements of the approach and their significance are also discussed.
Gruebele Martin
Roberts Gareth
Zewail Ahmed H.
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