Exploration of Coulomb explosion dynamics through excited vibrational states of molecules

Details Exploration of Coulomb explosion dynamics through excited vibrational states of molecules Exploration of Coulomb explosion dynamics through excited vibrational states of molecules

Jan 2005

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2005phrva..71a1402z&link_type=abstract

Physical Review A, vol. 71, Issue 1, id. 011402

Physics

1

Strong-Field Excitation Of Optical Transitions In Quantum Systems, Multiphoton Processes, Dynamic Stark Shift, Multiphoton Ionization And Excitation To Highly Excited States, Electronic Excitation And Ionization Of Molecules, Intermediate Molecular States

Scientific paper

The fragmentation dynamics of H+2 molecular ions in intense laser fields is investigated by means of a high-precision ab initio method beyond the Born-Oppenheimer approximation. Special attention is paid to the detailed Coulomb explosion (CE) mechanisms and dynamics through excited vibrational states of H+2 . A kinetic-energy release (KER) spectrum and CE phenomenon is predicted, in which the kinetic-energy distribution of H+ ions exhibits a series of peaks separated by one photon energy. A proposed scheme for observation of the KER spectrum and CE dynamics is presented.

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