Entangling remote nuclear spins linked by a chromophore

Details Entangling remote nuclear spins linked by a chromophore Entangling remote nuclear spins linked by a chromophore

2009-11-27

arxiv.org/abs/0911.5320v4

Phys. Rev. Lett. 104, 200501 (2010)

Physics

Quantum Physics

Scientific paper

10.1103/PhysRevLett.104.200501

Molecular nanostructures may constitute the fabric of future quantum technologies, if their degrees of freedom can be fully harnessed. Ideally one might use nuclear spins as low-decoherence qubits and optical excitations for fast controllable interactions. Here, we present a method for entangling two nuclear spins through their mutual coupling to a transient optically-excited electron spin, and investigate its feasibility through density functional theory and experiments on a test molecule. From our calculations we identify the specific molecular properties that permit high entangling power gates under simple optical and microwave pulses; synthesis of such molecules is possible with established techniques.

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