Electrochemical studies of copper and lead complexation by fulvic acid. I. Potentiometric measurements and a critical comparison of metal binding models

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Copper and lead ion-selective electrodes have been used to monitor titrations of Pb and Cu with fulvic acid extracted from the River Tamar, Southwest England. The titrations were carried out in 0.1 M NaClO 4 at 25°C at pH values in the range 6.0 to 6.5. The titration data were analysed using five different models; two assuming small values of discrete binding sites (multi-site and multidendate models), and three assuming continua of binding sites (electrostatic, normal distribution and affinity spectrum models). On both statistical and practical grounds the multi-site model was identified as the most effective in modelling the data. A synthetic data set proposed by and (1984) was used to examine the effect of random errors on the various data analysis procedures.

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