Development of Femtosecond Stimulated Raman Spectroscopy as a Probe of Vibrational Dynamics

Details Development of Femtosecond Stimulated Raman Spectroscopy as a Probe of Vibrational Dynamics Development of Femtosecond Stimulated Raman Spectroscopy as a Probe of Vibrational Dynamics

Jun 2011

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2011mss..confere04k&link_type=abstract

"International Symposium On Molecular Spectroscopy, 66th Meeting, Held 20-24 June, 2011 at Ohio State University. http://molspec

Physics

Dynamics

Scientific paper

Femtosecond stimulated Raman spectroscopy (FSRS) has proven to be a reliable probe of condensed phase dynamics by simultaneously achieving both exceptional temporal and frequency resolution. We report on preliminary attempts to utilize FSRS as a probe of vibrational relaxation on the ground electronic state of cyclohexane. We implement a 400 nm Raman pump/probe process following an IR actinic pump pulse which excites the C-H stretch overtone. Progress toward the use of FSRS as a tool alongside transient absorption measurements in vibrationally mediated photoisomerization experiments will also be discussed.

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