Control and imaging of single-molecule spectral dynamics using a nano-electrode

Details Control and imaging of single-molecule spectral dynamics using a nano-electrode Control and imaging of single-molecule spectral dynamics using a nano-electrode

2009-06-09

arxiv.org/abs/0906.1624v1

Molecular Physics, Volume 107, Issue 18, January 2009 , pages 1975 - 1979

Physics

Chemical Physics

5 pages, 4 figures

Scientific paper

10.1080/00268970903188358

We study the influence of a scanning nano-electrode on fluorescence excitation spectra of single terrylene molecules embedded in thin p-terphenyl films at cryogenic temperatures. We show that applied voltages less than 10 V can result in reversible Stark shifts of up to 100 times and linewidth increase greater than 10 times the natural linewidth. We discuss the potential of our experimental scheme for direct imaging of individual two-level systems (TLS) in the nanometer vicinity of single molecules.

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