Condensation of HNO3 on falling ice particles - Mechanism for denitrification of the polar stratosphere

Physics

Scientific paper

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Atmospheric Composition, Ice Clouds, Nitric Acid, Polar Meteorology, Stratosphere, Atmospheric Models, Atmospheric Temperature, Cooling, Evaporation, Particle Size Distribution

Scientific paper

Ice particles created in polar stratospheric cooling events are predicted to descend into Type I PSCs and accrete a coating of nitric acid trihydrate (NAT) that inhibits evaporation. Coated particles efficiently strip HNO3 from the atmosphere, providing a mechanism for denitrification without significant dehydration. Coatings that disintegrate may release large particles of NAT that influence subsequent particle growth.

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