Competitive oxidation in atmospheric aerosols: The case for relative kinetics

Details Competitive oxidation in atmospheric aerosols: The case for relative kinetics Competitive oxidation in atmospheric aerosols: The case for relative kinetics

Aug 2005

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2005georl..3216805d&link_type=abstract

Geophysical Research Letters, Volume 32, Issue 16, CiteID L16805

Physics

4

Atmospheric Composition And Structure: Aerosols And Particles (0345, 4801, 4906), Atmospheric Composition And Structure: Chemical Kinetic And Photochemical Properties, Atmospheric Composition And Structure: Pollution: Urban And Regional (0305, 0478, 4251), Atmospheric Composition And Structure: Troposphere: Composition And Chemistry

Scientific paper

We develop relative kinetics for heterogeneous oxidation of multi-component organic aerosols. Common accommodation, diffusion, and deposition terms cancel in this formulation, and rate constants may be determined for many compounds simultaneously within an aerosol with a realistic composition. Finally, cross-phase relative rate constants with a gas-phase reference compound and a condensed-phase target compound provide effective rate constants for use in atmospheric models.

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