Coherent Optimal Control of Multiphoton Molecular Excitation

Details Coherent Optimal Control of Multiphoton Molecular Excitation Coherent Optimal Control of Multiphoton Molecular Excitation

2003-06-24

arxiv.org/abs/physics/0306173v1

Journal of Physics B, 34, page 2189, 2001

Physics

Chemical Physics

5 figures

Scientific paper

10.1088/0953-4075/34/11/311

We give a framework for molecular multiphoton excitation process induced by an optimally designed electric field. The molecule is initially prepared in a coherent superposition state of two of its eigenfunctions. The relative phase of the two superposed eigenfunctions has been shown to control the optimally designed electric field which triggers the multiphoton excitation in the molecule. This brings forth flexibility in desiging the optimal field in the laboratory by suitably tuning the molecular phase and hence by choosing the most favorable interfering routes that the system follows to reach the target. We follow the quantum fluid dynamical formulation for desiging the electric field with application to HBr molecule.

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