Coherent control of nuclear spin isomers of molecules: The role of molecular motion

Physics – Chemical Physics

Scientific paper

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REVTEX, 13 pages + 3 eps figures

Scientific paper

10.1080/00268970110117755

Molecular center-of-mass motion is taken into account in the theory of
coherent control of nuclear spin isomers of molecules. It is shown that
infrared radiation resonant to the molecular rovibrational transition can
substantially enrich nuclear spin isomers and speed up their conversion rate.

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