Coherent Control of Isotope Separation in HD+ Photodissociation by Strong Fields

Details Coherent Control of Isotope Separation in HD+ Photodissociation by Strong Fields Coherent Control of Isotope Separation in HD+ Photodissociation by Strong Fields

1995-08-22

arxiv.org/abs/chem-ph/9508003v2

Physics

Chemical Physics

Physical Review Letters, 1995 (in press). 4 pages in revtex format, 3 uuencoded figures. Full postcript version available at:

Scientific paper

10.1103/PhysRevLett.75.2815

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent superposition of the fundamental radiation with its second harmonic can lead to asymmetries in the fragment angular distributions, with significant differences between the hydrogen and deuterium distributions in the long wavelength domain where the permanent dipole is most efficient. This effect is used to induce an appreciable isotope separation.

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