Coherent control of enrichment and conversion of molecular spin isomers

Details Coherent control of enrichment and conversion of molecular spin isomers Coherent control of enrichment and conversion of molecular spin isomers

2000-11-05

arxiv.org/abs/physics/0011012v1

Phys. Rev. A v.63, 063402-(1-7) (2001)

Physics

Chemical Physics

REVTEX, 13 pages + 6 eps figures

Scientific paper

10.1103/PhysRevA.63.063402

A theoretical model of nuclear spin conversion in molecules controlled by an external electromagnetic radiation resonant to rotational transition has been developed. It has been shown that one can produce an enrichment of spin isomers and influence their conversion rates in two ways, through coherences and through level population change induced by radiation. Influence of conversion is ranged from significant speed up to almost complete inhibition of the process by proper choice of frequency and intensity of the external field.

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