Classical-Wigner Phase Space Approximation to Cumulative Matrix Elements in Coherent Control

Details Classical-Wigner Phase Space Approximation to Cumulative Matrix Elements in Coherent Control Classical-Wigner Phase Space Approximation to Cumulative Matrix Elements in Coherent Control

2003-05-30

arxiv.org/abs/physics/0305132v1

J. Chem. Phys. 119, 3606 (2003).

Physics

Chemical Physics

17 pages, 12 figures, to appear in Journal of Chemical Physics

Scientific paper

10.1063/1.1590962

The classical limit of the Wigner-Weyl representation is used to approximate products of bound-continuum matrix elements that are fundamental to many coherent control computations. The range of utility of the method is quantified through an examination of model problems, single-channel Na_2 dissociation and multi-arrangement channel photodissociation of CH_2IBr. Very good agreement with the exact quantum results is found for a wide range of system parameters.

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