Charge transfer dynamics in driven molecular ratchets: quantum Monte Carlo results and rate models

Details Charge transfer dynamics in driven molecular ratchets: quantum Monte Carlo results and rate models Charge transfer dynamics in driven molecular ratchets: quantum Monte Carlo results and rate models

Mar 2009

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2009njph...11c5001m&link_type=abstract

New Journal of Physics, Volume 11, Issue 3, pp. 035001 (2009).

Physics

4

Scientific paper

Charge transfer dynamics is studied in a ratchet-type molecular wire subject to finite frequency driving. Numerically exact data are obtained within the path integral Monte Carlo approach over the full transient time regime until a stationary net population imbalance has been established. This allows for a quantitative comparison with the master equation approaches and, in particular, underlines the usefulness of these rate models.

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