Bending-induced diminution of shape resonances in the core-level absorption region of hot CO2 and N2O

Details Bending-induced diminution of shape resonances in the core-level absorption region of hot CO2 and N2O Bending-induced diminution of shape resonances in the core-level absorption region of hot CO2 and N2O

Dec 2010

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2010njph...12l3017t&link_type=abstract

New Journal of Physics, Volume 12, Issue 12, pp. 123017 (2010).

Physics

Scientific paper

We have measured the initial vibrational-state-specific, symmetry-resolved ion-yield spectra of CO2 and N2O in the shape resonance regions above the K-shell ionization thresholds. For both molecules, significant diminution of the shape resonances by bending excitation in the initial electronic ground state is observed. The measured ion-yield spectra are well reproduced by calculations employing the Schwinger variational principle. The observed changes in the spectra are seen to be due to a shift of the resonances to lower energy and an initial increase in width with bending.

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