Analysis of the Magnetic Hyperfine Structure in the B^{3}Φ_{4}-X^{3}Φ_{4} Band System of Iridium Monofluoride, IrF

Details Analysis of the Magnetic Hyperfine Structure in the B^{3}Φ_{4}-X^{3}Φ_{4} Band System of Iridium Monofluoride, IrF Analysis of the Magnetic Hyperfine Structure in the B^{3}Φ_{4}-X^{3}Φ_{4} Band System of Iridium Monofluoride, IrF

Jun 2009

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2009mss..conferf04w&link_type=abstract

"International Symposium On Molecular Spectroscopy, 64th Meeting, Held 22-26 June, 2009 at Ohio State University. http://molspec

Physics

Electronic

Scientific paper

Recently the New Brunswick group reported on the detection and analysis of the B^{3}Φ_{4}-X^{3}Φ_{4} band system of IrF. The free-jet expansion conditions limited the spectral resolution to approximately 200 MHz, which was insufficient to fully resolve the ^{191}Ir(I=3/2), ^{193}Ir(I=3/2)and ^{19}F(I=1/2)magnetic hyperfine splitting. Here we report on the analysis of the same band system recorded under molecular beam conditions which resulted in a resolution of 40 MHz. A simple molecular orbital correlation diagram is used to rationalize the determined parameters of IrF and the isovalent molecules RhF and CoF.
A.G. Adam; A.D. Granger; L.E. Downie; D.W. Tokaryk and C. Linton Can.J. Phys. (accepted).
R. Li, R.J. Jensen, W.J. Balfour, S.A. Shepard and A.G. Adam; J.Chem.Phys. 121 2591, 2004.
J.J. Harrison, J.M. Brown, M.A. Flory, P.M. Sheridan, S.K. McLamarrah and L.M. Ziurys J. Chem. Phys. 127 194308, 2007.

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