An Implementation of the Deutsch-Jozsa Algorithm on Molecular Vibronic Coherences Through Four-Wave Mixing: a Theoretical Study

Details An Implementation of the Deutsch-Jozsa Algorithm on Molecular Vibronic Coherences Through Four-Wave Mixing: a Theoretical Study An Implementation of the Deutsch-Jozsa Algorithm on Molecular Vibronic Coherences Through Four-Wave Mixing: a Theoretical Study

2001-10-06

arxiv.org/abs/quant-ph/0110041v4

Chem. Phys. Lett. 360, 459 (2002)

Physics

Quantum Physics

Replaced with published version. 14 pages, 2 figures, 1 table

Scientific paper

10.1016/S0009-2614(02)00808-4

Time-Frequency Resolved Coherent Anti-Stokes Raman Scattering (TFRCARS) was recently proposed as a means to implement quantum logic using the molecular ro-vibrational manifold as a quantum register [R. Zadoyan et al., Chem. Phys. 266, 323 (2001)]. We give a concrete example of how this can be accomplished through an illustrative algorithm that solves the Deutsch-Jozsa problem. We use realistic molecular parameters to recognize that, as the problem size expands, shaped pulses must be tailored to maintain fidelity of the algorithm.

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