A general algebraic model for molecular vibrational spectroscopy

Details A general algebraic model for molecular vibrational spectroscopy A general algebraic model for molecular vibrational spectroscopy

1996-04-11

arxiv.org/abs/chem-ph/9604005v1

Ann. Phys. (N.Y.) 252 (1996) 211

Physics

Chemical Physics

35 pages TEX, submitted to Annals of Physics (N.Y.)

Scientific paper

10.1006/aphy.1996.0129

We introduce the Anharmonic Oscillator Symmetry Model to describe vibrational excitations in molecular systems exhibiting high degree of symmetry. A systematic procedure is proposed to establish the relation between the algebraic and configuration space formulations, leading to new interactions in the algebraic model. This approach incorporates the full power of group theoretical techniques and provides reliable spectroscopic predictions. We illustrate the method for the case of ${\cal D}_{3h}$-triatomic molecules.

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