A determination of the rate constant for the reaction of HOCL with O-atoms at room temperature

Details A determination of the rate constant for the reaction of HOCL with O-atoms at room temperature A determination of the rate constant for the reaction of HOCL with O-atoms at room temperature

Oct 1992

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1992georl..19.1935v&link_type=abstract

Geophysical Research Letters (ISSN 0094-8276), vol. 19, no. 19, p. 1935-1937.

Physics

5

Atmospheric Chemistry, Chlorine Oxides, Oxygen Atoms, Photochemical Reactions, Reaction Kinetics, Free Radicals, Mass Spectrometers, Room Temperature

Scientific paper

A discharge fast flow system with mass spectrometric detection was used to determine the rate constant of the title reaction to be k(1) = (1.3 +/- 0.2) x 10 exp -13 cu cm/molecule/s. This experimental value is roughly a factor of 20 higher than previously recommended. It is suggested that the title reaction should be considered as a removal process in modeling stratospheric HOCl.

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