Comparison of experiments and theory in time resolved fluorescence spectroscopy

Physics – Optics

Scientific paper

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Scientific paper

The time dependent fluorescence of mercury atoms that were excited by short pulses of electrons or laser light to the 6 3P1 state can be explained by a theoretical approach which describes the fluorescent light as a sum I(t) = Σ∞n=0Sn where Sn is the signal due to those photons that have been reabsorbed and reemitted n-times before leaving the experimental geometry. Measurements using different isotopes of a mercury sample can be reproduced theoretically for two of the isotopes with no additional free parameter, if one parameter (absorption coefficient) is fitted to the signal of the third isotope.

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