Impact of stratospheric ozone recovery on tropospheric ozone and its budget

Physics

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Atmospheric Composition And Structure: Troposphere: Composition And Chemistry, Atmospheric Composition And Structure: Troposphere: Constituent Transport And Chemistry, Global Change: Impacts Of Global Change (1225), Atmospheric Composition And Structure: Evolution Of The Atmosphere (1610, 8125)

Scientific paper

We consider the impact of stratospheric ozone recovery between 2000 and 2100 on modeled tropospheric ozone and the tropospheric ozone budget, using a tropospheric chemistry-climate model. Ozone calculated from a stratospheric chemistry-climate model is used to prescribe lower stratospheric ozone in the tropospheric model. The results show that stratospheric ozone recovery leads to significant increases of tropospheric ozone throughout the extra-tropical troposphere, in particular, a large surface ozone increase in the Southern Hemisphere during austral winter months. Stratospheric ozone recovery and climate change contribute about equally to the increase in surface ozone during this season.

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