Vibrational interference of Raman and high-harmonic generation pathways

Details Vibrational interference of Raman and high-harmonic generation pathways Vibrational interference of Raman and high-harmonic generation pathways

2009-08-06

arxiv.org/abs/0908.0896v1

Physics

Atomic Physics

Scientific paper

Experiments have shown that the internal vibrational state of a molecule can affect the intensity of high harmonic light generated from that molecule. This paper presents a model which explains this modulation in terms of interference between different vibrational states occurring during the high harmonic process. In addition, a semiclassical model of the continuum electron propagation is developed which connects with rigorous treatments of the electron-ion scattering.

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