Orientation of molecules via laser-induced anti-alignment

Physics – Quantum Physics

Scientific paper

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Scientific paper

10.1103/PhysRevA.73.061401

We show that field-free molecular orientation induced by a half-cycle pulse
may be considerably enhanced by an additional laser pulse inducing molecular
anti-alignment. Two qualitatively different enhancement mechanisms are
identified depending on the pulse order, and their effects are optimized with
the help of quasi-classical as well as fully quantum models.

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