Non-adiabatic coupling and adiabatic population transfer in quantum molecular systems

Details Non-adiabatic coupling and adiabatic population transfer in quantum molecular systems Non-adiabatic coupling and adiabatic population transfer in quantum molecular systems

2002-03-15

arxiv.org/abs/physics/0203049v1

Physics

Chemical Physics

5 pages, 2 figures

Scientific paper

We show that a counter-intuitive pulse sequence leads to adiabatic passage
between the vibrational levels of three harmonic potentials through parallel
dark states in adiabatic approximation. However, the adiabatic assumptions
break down for very intense pulses and non-adiabatic couplings result in the
population transfer by light-induced potential shaping.

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