Delayed optical nonlinearity of thin metal films

Details Delayed optical nonlinearity of thin metal films Delayed optical nonlinearity of thin metal films

2011-09-27

arxiv.org/abs/1109.5875v1

Physics

Optics

Scientific paper

Metals typically have very large nonlinear susceptibilities, whose origin is
mainly of thermal character. We model the cubic nonlinearity of thin metal
films by means of a delayed response derived \textit{ab initio} from an
improved version of the classic two temperature model. We validate our model by
comparison with ultrafast pump-probe experiments on gold films.

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