Theory for Diffusion-Limited Oscillating Chemical Reactions

Details Theory for Diffusion-Limited Oscillating Chemical Reactions Theory for Diffusion-Limited Oscillating Chemical Reactions

1996-12-12

arxiv.org/abs/physics/9612008v2

J. Stat. Phys. 87, 1165-1178 (1997)

Physics

Chemical Physics

16 pages, 4 figures, final version as published

Scientific paper

10.1007/BF02181278

A kinetic description of lattice-gas automaton models for reaction-diffusion systems is presented. It provides corrections to the mean-field rate equations in the diffusion-limited regime. When applied to the two-species Maginu model, the theory gives an excellent quantitative prediction of the effect of slow diffusion on the periodic oscillations of the average concentrations in a spatially homogeneous state.

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