On multiphoton absorption by molecules

Details On multiphoton absorption by molecules On multiphoton absorption by molecules

1998-03-17

arxiv.org/abs/quant-ph/9803043v1

Physics

Quantum Physics

4 pages, RevTex, to appear in Theochem

Scientific paper

Rabi frequencies for multiphoton absorption by atoms or molecules that can be characterized as two- or three-level systems are obtained in the cases of single and double laser perturbations. If the ambiguity in the origin of absolute energy is conveniently gauged off in the three-level model, there appears an additional non linear frequency which is originated from the separate evolution of a relative-frequency component induced in the whole system by the simultaneous action of the two perturbations.

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