Physics – Chemical Physics
Scientific paper
1996-03-31
Chem. Phys. Lett. 255, 309 1996
Physics
Chemical Physics
RevTeX in LaTeX file, 12 preprint pages, 4 ps figures included. Also available from http://insti.physics.sunysb.edu/~mmartin/p
Scientific paper
10.1016/0009-2614(96)00388-0
Molecular dynamics calculations and optical spectroscopy measurements of weakly active infrared modes are reported. The results are qualitatively understood in terms of the "motional diminishing" of IR lines, a process analogous to the motional narrowing of a nuclear magnetic resonance (NMR) signal. In molecular solids or liquids where the appropriate intramolecular resonances are observable, motional diminishing can be used to study the fluctuations of the intermolecular interactions having time scales of 1psec to 100psec.
Martin Michael C.
Mihaly Laszlo
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