Laser-induced fluorescence spectroscopy of the Hg3 excimer

Details Laser-induced fluorescence spectroscopy of the Hg3 excimer Laser-induced fluorescence spectroscopy of the Hg3 excimer

Sep 1986

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1986phrva..34.2483n&link_type=abstract

Physical Review A - General Physics, 3rd Series (ISSN 0556-2791), vol. 34, Sept. 1986, p. 2483-2485. NSERC-supported research.

Physics

General Physics

7

Laser Induced Fluorescence, Laser Pumping, Laser Spectroscopy, Mercury (Metal), Metal Vapor Lasers, Excimer Lasers, Molecular Energy Levels, Spectral Bands, Temporal Distribution, Ultraviolet Spectra, Fluorescence And Phosphorescence Spectra

Scientific paper

The first observation of a laser-induced fluorescence band, excited by absorption from a low-lying state of the Hg3 excimer using a 'pump-and-probe' method, is reported. A study of the fluorescence intensity as a function of the time separation between the 'pump' and 'probe' laser pulses provides clear evidence for the presence of both Hg3 and Hg2 molecules in the laser-excited mercury vapor. The fluorescence may be due to trimer emission or to dimer emission following dissociation of a trimer state.

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