Rate constants for the reactions of CO3-(H2O)n=0-5+SO2: Implications for CIMS detection of SO2

Details Rate constants for the reactions of CO3-(H2O)n=0-5+SO2: Implications for CIMS detection of SO2 Rate constants for the reactions of CO3-(H2O)n=0-5+SO2: Implications for CIMS detection of SO2

Jun 1997

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1997georl..24.1379s&link_type=abstract

Geophysical Research Letters, Volume 24, Issue 11, p. 1379-1382

Physics

9

Atmospheric Composition And Structure, Atmospheric Composition And Structure: Chemical Kinetic And Photochemical Properties, Atmospheric Composition And Structure: Ion Chemistry Of The Atmosphere, Atmospheric Composition And Structure: Instruments And Techniques

Scientific paper

The rate constants for the CO3-(H2O)n+SO2 reactions were measured for n=0-5 using a variable temperature-selected ion flow tube. Temperature dependences were measured for n=0-3 over the following temperature ranges: n=1, 158-550 K; n=1, 158-270 K; n=2, 158-193 K; n=3, 158-193. The n=4, 5 rate constants were measured exclusively at 158 K. Good agreement is found with previous measurements of the n=0 and 1 rate constants. Expressions are estimated for use in chemical ionization mass spectrometric detection of SO2 in the troposphere.

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